Spectrum and low-energy gap in triangular quantum spin liquid NaYbSe2

Abstract: 

We report neutron scattering, pressure-dependent AC calorimetry, and AC magnetic susceptibility measurements of triangular lattice NaYbSe2. We observe a continuum of scattering, which is reproduced by matrix product simulations, and no phase transition is detected in any bulk measurements. Comparison to heat capacity simulations suggest the material is within the Heisenberg spin liquid phase. AC Susceptibility shows a significant 23~mK downturn, indicating a gap in the magnetic spectrum. The combination of a gap with no detectable magnetic order, comparison to theoretical models, and comparison to other AYbSe2 compounds all strongly indicate NaYbSe2 is within the quantum spin liquid phase. The gap also allows us to rule out a gapless Dirac spin liquid, with a gapped 2 liquid the most natural explanation.

Author: 
Scheie AO
Lee M
Wang K
Laurell P
Choi ES
Pajerowski D
et al
Publication date: 
June 25, 2024
Publication type: 
Journal Article